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During this series Thor was slowly going insane and Valkyrie would ultimately manifest as Thor's insanity made flesh (more or less) - although female she was the embodiment of Thor's madness and fought against him and many other heroes during this event.
As the embodiment of Thor's own insanity Valkyrie shared a special bond with Thor and could corrupt the thunder-god with her presence, going as far as enslaving him to her will if she gained enough control over him.